| Faust |
Nikos Hadjinikolaou |
12, 14, 17, 19, 22 November & 10, 16 December 1959 / 8 January & 2 February & 3 March 1960 |
| Faust |
Giorgio Kokolios-Bardi |
24, 26 November 1959 |
| Faust |
Antonis Papakonstantinou |
25 February & 10 March 1960 |
| Mephistopheles |
Nicola Moscona |
12, 14, 17, 19, 22, 24 November 1959 |
| Mephistopheles |
Petros Hoidas |
10, 16 December 1959 / 8 January & 2, 25 February & 3, 10 March 1960 |
| Marguerite |
Zoe Vlachopoulos |
12, 14, 17, 19, 22 November 1959 / 2 February 1960 |
| Marguerite |
Tatiana Tsachouridou |
24, 26 November & 10, 16 December 1959 / 8 January 1960 |
| Marguerite |
Flora Kazatzian |
25 February & 3, 10 March 1960 |
| Valentin |
Wassili Janulako |
12, 14, 17, 19, 22, 24 November & 10, 16 December 1959 / 8 January & 3, 10 March 1960 |
| Valentin |
Manuel Ausensi |
2, 25 February 1960 |
| Wagner |
Yorgos Zakkas |
12, 14, 17, 19, 22, 24 November & 10, 16 December 1959 / 8 January & 2, 25 February & 3, 10 March 1960 |
| Wagner |
Tzanetos Doukakos |
26 November 1959 |
| Siébel |
Tatiana Tsachouridou |
12, 14, 17, 19, 22 November 1959 / 10 March 1960 |
| Siébel |
Eva Delazanou |
24, 26 November & 10, 16 December 1959 / 8 January & 2, 25 February & 3 March 1960 |
| Marta |
Kiki Morfoniou-Komisopoulou |
12, 14, 17, 19, 22, 24, 26 November & 10, 16 December 1959 / 8 January & 2, 25 February & 3, 10 March 1960 |