| Faust |
Doro (Isidoro) Antonioli |
21, 26, 30 June & 3, 7 July 1963 |
| Faust |
Nikos Hadjinikolaou |
23 June 1963 |
| Mephistopheles |
Nicola Moscona |
21, 23, 26, 30 June & 3, 7 July 1963 |
| Marguerite |
Tatiana Tsachouridou |
21, 23, 26, 30 June 1963 |
| Marguerite |
Flora Kazatzian |
3, 7 July 1963 |
| Valentin |
Kostas Paskalis |
21, 23 June & 3, 7 July 1963 |
| Valentin |
Kostis Dimitrakopoulos |
26 June 1963 |
| Valentin |
John (Ioannis Philippos) Modinos |
30 June 1963 |
| Wagner |
Yorgos Zakkas |
21, 23, 26, 30 June & 3, 7 July 1963 |
| Siébel |
Nana Goutou-Mog |
21, 23, 26, 30 June & 3, 7 July 1963 |
| Marta |
Anna Maragaki |
21, 23, 26, 30 June & 3, 7 July 1963 |