| Mephistopheles |
Raffaele Arie |
18, 20, 23, 27 November 1966 |
| Faust |
Luigi Ottolini |
18, 20, 23, 27 November 1966 |
| Marguerite |
Tatiana Tsachouridou |
18, 20, 23, 27 November 1966 |
| Marta |
Kiki Morfoniou-Komisopoulou |
18, 20 November 1966 |
| Marta |
Lela Stamos |
23, 27 November 1966 |
| Wagner |
Aristides Pantazinakos |
18, 20, 23, 27 November 1966 |
| Elena |
Soula Glantzi |
18, 20, 23, 27 November 1966 |
| Pantalis |
Lela Stamos |
18, 20, 23, 27 November 1966 |
| Nereo |
Lyssandros Ioannidis |
18, 20, 23, 27 November 1966 |
